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Abstract

The resonance lifetime and energy of an excited Cs-state on Cu(111)
M. Bauer, S. Pawlik, M. Aeschlimann
Phys. Rev. B. 55 (1997) 10040


Using time-resolved two-photon photoemission spectroscopy, we investigated the resonance lifetime and energy of an excited Cs-state on Cu(111) in the low-coverage case. We found a pronounced lifetime increase of up to 11 3fs on a copper surface covered with cesium as compared to a clean copper surface in the energy range of an excited electronic Cs-state in the spectrum. This result is in agreement with recent theoretical predictions of hybridization among excited atomic levels of alkali atoms near metal surfaces.

PACS numbers: 70.60.B, 78.47, 79.60

 

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